TIME-RESOLVED DARK-FIELD X-RAY MICROSCOPY

Revealing Defect-Mediated Lattice Dynamics with Time-Resolved Dark-Field X-ray Microscopy

Time-resolved DFXM images how a laser-induced strain field propagates and undergoes mode conversion upon interacting with defects.
The high penetration depth of X-rays enables subsurface wave components to be tracked throughout the bulk.

Seong Gook KimPOSTECH · Max Planck POSTECH/Korea Research Initiative

EXPERIMENTAL DATA

Movies

01

Overall pump–probe experiment

This movie summarizes the full time-resolved DFXM measurement sequence. Periodic intact-state measurements were interleaved with the pump–probe delay scans to verify reversible sample recovery and measurement reproducibility.

02–1

Representative case: annotated wave propagation

Blue arrows indicate the longitudinal strain wave propagating along the depth direction, while red arrows indicate the transverse elastic wave propagating in plane.

02–2

Larger-beam case: extended field of view

A larger beam size enables a broader sample region to be probed. Consistent longitudinal and transverse wave responses are also observed near the dislocation on the right; the red arrows specifically mark the transverse in-plane component.

02–3

Weak-contrast dislocation case: transverse-wave response

The same in-plane transverse strain-wave response is observed at a weak-contrast dislocation from 1,000 to 6,000 ps. The red arrow marks its propagation.

SUPPLEMENTARY MATERIAL

Supplementary figures

Swipe through the analysis—from ultrafast excitation to strain-wave propagation.

Ge dislocation geometries alongside their corresponding DFXM difference images
01 · DEFECT CONTRAST

Ge {111}⟨110⟩ dislocations

In our experimental geometry, the DFXM contrast and its characteristic image shape depend on the dislocation type and orientation. The difference images are obtained by subtracting the perfect-crystal DFXM image from the defect-containing case.

Simulated DFXM response to lateral translation of a localized strain field Simulated DFXM response to inward translation of a localized strain field
02 · DFXM SIMULATION

Simulated DFXM response to strain translation

To model strain-wave propagation, a localized strain field was translated laterally and inward; the resulting DFXM contrast shifts agree with geometric predictions and do not represent physical defect motion.

Calculated electron and lattice temperatures as a function of time
03 · TTM SIMULATION

Electronic and lattice temperature response

COMSOL two-temperature-model simulation of ultrafast laser excitation in germanium, showing rapid electron heating followed by electron–phonon energy transfer to the lattice.

Stacked profiles annotated with in-plane and out-of-plane wave components and the initial defect position
04 · OVERVIEW

Overall DFXM dynamics

Stacked DFXM profiles show the overall evolution of the out-of-plane longitudinal and in-plane transverse strain-wave components.